In order to solve the problem of a thin deposition layer on the titanium alloy in the traditional friction surfacing process of dissimilar Ti/Al metals, new shoulder-restricted friction deposition (SRFD) equipment was successfully developed by introducing a restricted shoulder. Using a laser to roughen the titanium substrate, the process verification of Al deposition onto TC4 was realized. The material utilization was close to 100%, and a deposition layer with a thickness of 0.8 mm and a strong bonded interface was obtained. The peel strength of the triple-layer deposited joints was 121 MPa.